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This research demonstrates a novel method for coherent quantum control by exploiting interference between second- and third-order nonlinear optical processes, enabling precise shaping of biphoton wavefunctions without classical analogues. By integrating these distinct generation mechanisms—spontaneous parametric down-conversion and four-wave mixing—onto a single photonic platform, the study advances fundamental capabilities in quantum nonlinear optics essential for scalable quantum information processing.
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Coherent control of photon pairs via quantum interference between second- and third-order quantum nonlinear processes

arXiv2 min read

arXiv:2601.18746v2 Announce Type: replace-cross Abstract: Genuine quantum interference between independent nonlinear processes of different order provides a route to coherent control that cannot be reduced to a classical field interference. Here we present an all-optical analogue of coherent carrier injection by exploiting interference between second- and third-order quantum nonlinear processes in an integrated photonic platform. Photon pairs generated via spontaneous parametric down-conversion and spontaneous four-wave mixing coherently contribute to the same final two-photon state, resulting in a phase-dependent modulation of both the generation rate and the spectral structure of the emitted biphoton state. We illustrate the features of such interference and how it can be used to shape biphoton wavefunctions and their quantum correlations. These results identify interference between nonlinear processes of different order as a distinct form of coherent quantum control within quantum nonlinear optics.

Abstract:Genuine quantum interference between independent nonlinear processes of different order provides a route to coherent control that cannot be reduced to a classical field interference. Here we present an all-optical analogue of coherent carrier injection by exploiting interference between second- and third-order quantum nonlinear processes in an integrated photonic platform. Photon pairs generated via spontaneous parametric down-conversion and spontaneous four-wave mixing coherently contribute to the same final two-photon state, resulting in a phase-dependent modulation of both the generation rate and the spectral structure of the emitted biphoton state. We illustrate the features of such interference and how it can be used to shape biphoton wavefunctions and their quantum correlations. These results identify interference between nonlinear processes of different order as a distinct form of coherent quantum control within quantum nonlinear optics.

Optics (physics.optics); Quantum Physics (quant-ph)

arXiv:2601.18746 [physics.optics]

(or arXiv:2601.18746v2 [physics.optics] for this version)

https://doi.org/10.48550/arXiv.2601.18746 Focus to learn more arXiv-issued DOI via DataCite

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Full text under the publisher's open licence · 225 words

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