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This research addresses the fundamental challenge of energy trapping in dark states within optical microcavity systems by utilizing non-Condon exciton-phonon coupling to create a one-way escape route into radiative channels. The proposed mechanism achieves near-complete transport efficiency independent of system size, offering significant potential for optimizing light harvesting and dissipation-based quantum control protocols. By recasting parasitic loss modes as an engineered resource, this work advances the theoretical framework for scalable polariton transport networks.
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Unidirectional Dark-to-Bright Rescue in Cavity-Coupled Quantum Transport

arXiv2 min read

arXiv:2608.05312v1 Announce Type: new Abstract: Strong light-matter coupling in optical microcavities can transport energy ballistically across an emitter array, but the same coupling buries most of the excitation in a manifold of dark states that grows with system size and traps energy outside the transport channel. We show that the off-diagonal (non-Condon) part of the exciton-phonon coupling opens a one-way escape route from this trap, driving population irreversibly from dark states into the radiative channel. This rate is fixed by a photonic-weight conservation law rather than by dark-bright overlap which evacuates the dark manifold at a rate independent of system size. The mechanism contributes to transport with near-complete efficiency with four signatures being single exponential dark state decay, a size scaling efficiency gap, distinct temperature behavior, and a resonance in the escape rate at vibrational bath modes. Beyond polariton transport, it recasts dark states from a parasitic loss channel into an engineered dissipative resource, with implications for light harvesting and dissipation based quantum control.

Abstract:Strong light-matter coupling in optical microcavities can transport energy ballistically across an emitter array, but the same coupling buries most of the excitation in a manifold of dark states that grows with system size and traps energy outside the transport channel. We show that the off-diagonal (non-Condon) part of the exciton-phonon coupling opens a one-way escape route from this trap, driving population irreversibly from dark states into the radiative channel. This rate is fixed by a photonic-weight conservation law rather than by dark-bright overlap which evacuates the dark manifold at a rate independent of system size. The mechanism contributes to transport with near-complete efficiency with four signatures being single exponential dark state decay, a size scaling efficiency gap, distinct temperature behavior, and a resonance in the escape rate at vibrational bath modes. Beyond polariton transport, it recasts dark states from a parasitic loss channel into an engineered dissipative resource, with implications for light harvesting and dissipation based quantum control.

arXiv:2608.05312 [quant-ph]

(or arXiv:2608.05312v1 [quant-ph] for this version)

https://doi.org/10.48550/arXiv.2608.05312 Focus to learn more arXiv-issued DOI via DataCite (pending registration)

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Full text under the publisher's open licence · 250 words

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