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This study establishes a diagnostic method using polarization-resolved photon statistics ($g^{(2)}$) to directly probe light-matter coupling and extract magnetic symmetries in quantum materials. By linking photon bunching patterns to matter correlation functions, the research provides a practical tool for characterizing phase transitions in systems like the Kitaev-Heisenberg spin model. The approach offers a novel pathway to isolate higher-order scattering processes, advancing the experimental toolkit for strongly correlated electron systems.
Polarization-Resolved Photon Statistics of Cavity Quantum Materials
arXiv:2606.11550v1 Announce Type: cross Abstract: By forming hybrid light-matter states, optical cavities offer a route for engineering material properties, however, unambiguously probing the effects of light-matter coupling remains difficult. Here, we show that the polarization-resolved statistics of photons transmitted through a cavity, measurable via $g^{(2)}$, provide one such diagnostic. By relating $g^{(2)}$ to matter correlation functions such as the Raman structure factor, we link photon bunching and antibunching to material properties. By applying this method to the stripy-to-antiferromagnetic transition in the Kitaev-Heisenberg spin model, we find that polarization-dependent patterns of bunching and antibunching encode the magnetic point-group symmetries of each phase and characterize the behavior at the phase boundary. Finally, we predict measuring $g^{(2)}$ for output photon pairs polarized orthogonal to the input field will isolate higher-order light-matter scattering processes that probe higher-order material correlations.
Abstract:By forming hybrid light-matter states, optical cavities offer a route for engineering material properties, however, unambiguously probing the effects of light-matter coupling remains difficult. Here, we show that the polarization-resolved statistics of photons transmitted through a cavity, measurable via $g^{(2)}$, provide one such diagnostic. By relating $g^{(2)}$ to matter correlation functions such as the Raman structure factor, we link photon bunching and antibunching to material properties. By applying this method to the stripy-to-antiferromagnetic transition in the Kitaev-Heisenberg spin model, we find that polarization-dependent patterns of bunching and antibunching encode the magnetic point-group symmetries of each phase and characterize the behavior at the phase boundary. Finally, we predict measuring $g^{(2)}$ for output photon pairs polarized orthogonal to the input field will isolate higher-order light-matter scattering processes that probe higher-order material correlations.
Mesoscale and Nanoscale Physics (cond-mat.mes-hall); Strongly Correlated Electrons (cond-mat.str-el); Optics (physics.optics); Quantum Physics (quant-ph)
arXiv:2606.11550 [cond-mat.mes-hall]
(or arXiv:2606.11550v1 [cond-mat.mes-hall] for this version)
https://doi.org/10.48550/arXiv.2606.11550 arXiv-issued DOI via DataCite (pending registration)
Full text under the publisher's open licence · 159 words
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