Tantalum as a base material for superconducting integrated circuits

Authors:Evgeniy V. Zikiy, Nikita S. Smirnov, Stanislav A. Kotenkov, Ilya A. Stepanov, Julia A. Agafonova, Daria A. Moskaleva, Aleksei R. Matanin, Anton I. Ivanov, Dmitry O. Moskalev, Julia A. Kurochkina, Aleksander V. Andriyash, Ilya A. Rodionov

Abstract:The performance of superconducting integrated circuits for quantum applications is fundamentally limited by material-related losses. Tantalum, as an emerging material for next-generation quantum circuits, has attracted considerable attention in recent years after demonstrating breakthrough performance in both superconducting microwave resonators and qubits. Concurrently, a growing body of work is devoted to the operation of tantalum-based circuits and related fabrication techniques. This interest is further stimulated by tantalum thin films polymorphism resulting in a variety of its crystalline structure, superconducting properties, coherence, etc. Furthermore, tantalum circuits exhibit distinctive features in cryogenic experiments, which have not been observed in aluminum- or niobium-based ones. In this review, we summarize the recent research of tantalum thin films growth and phase selection mechanisms on various substrates, key aspects of fabrication and performance of superconducting circuit, including a material first-principles theoretical study. In conclusion, we address a number of open issues, including the role of \b{eta}-phase impurities, the effect of hydrofluoric acid solutions on chain characteristics, and the anomalous behavior of {\alpha}-tantalum chains at cryogenic temperatures.

Quantum Physics (quant-ph); Materials Science (cond-mat.mtrl-sci)

arXiv:2606.13750 [quant-ph]

(or arXiv:2606.13750v1 [quant-ph] for this version)