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This research quantifies the resource overhead of teleportation-based distributed quantum computing for unitary coupled-cluster ansätze applied to hydrogen chains. By comparing naive distribution methods with the TeleSABRE algorithm, the study identifies that UpCCD circuits with spin-blocked Jordan-Wigner ordering offer superior scaling compared to UCCSD. These findings provide critical benchmarks for optimizing qubit connectivity and communication costs in scalable quantum chemistry simulations.
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Quantifying Teleportation Overhead in Distributed Unitary Coupled-Cluster Ans\"atze

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arXiv:2609.36266v1 Announce Type: new Abstract: Distributed quantum computing (DQC) has been proposed as a way to scale quantum algorithms for practical applications beyond monolithic quantum processor architectures. Among these applications, quantum chemistry is widely regarded as one of the most promising use cases for quantum computing. In this work, we estimate the distributed-resource requirements of unitary coupled-cluster (UCC) ans\"atze for quantum chemistry, focusing on unitary coupled-cluster singles and doubles (UCCSD), unitary pair coupled-cluster doubles (UpCCD), and unitary pair coupled-cluster with generalized singles and doubles (UpCCGSD) circuits for hydrogen chains. We focus on a teleportation-based approach to DQC, quantitatively comparing a naive distribution method to the output of the TeleSABRE algorithm. For both approaches, we estimate the cost of handling nonlocal two-qubit gates across a fixed midpoint or quarter-point partition, reporting Bell-pair/classical-communication costs in teleportation. Across Jordan-Wigner and Bravyi-Kitaev, we find that UpCCD with spin-blocked Jordan-Wigner ordering gives the most favorable scaling, while UCCSD incurs substantially larger distributed-resource requirements.

Abstract:Distributed quantum computing (DQC) has been proposed as a way to scale quantum algorithms for practical applications beyond monolithic quantum processor architectures. Among these applications, quantum chemistry is widely regarded as one of the most promising use cases for quantum computing. In this work, we estimate the distributed-resource requirements of unitary coupled-cluster (UCC) ansätze for quantum chemistry, focusing on unitary coupled-cluster singles and doubles (UCCSD), unitary pair coupled-cluster doubles (UpCCD), and unitary pair coupled-cluster with generalized singles and doubles (UpCCGSD) circuits for hydrogen chains. We focus on a teleportation-based approach to DQC, quantitatively comparing a naive distribution method to the output of the TeleSABRE algorithm. For both approaches, we estimate the cost of handling nonlocal two-qubit gates across a fixed midpoint or quarter-point partition, reporting Bell-pair/classical-communication costs in teleportation. Across Jordan-Wigner and Bravyi-Kitaev, we find that UpCCD with spin-blocked Jordan-Wigner ordering gives the most favorable scaling, while UCCSD incurs substantially larger distributed-resource requirements.

Quantum Physics (quant-ph); Distributed, Parallel, and Cluster Computing (cs.DC); Chemical Physics (physics.chem-ph)

arXiv:2609.36266 [quant-ph]

(or arXiv:2609.36266v1 [quant-ph] for this version)

https://doi.org/10.48550/arXiv.2609.36266 Focus to learn more arXiv-issued DOI via DataCite (pending registration)

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