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This research demonstrates a novel method for probing light-matter coupling in quantum materials by analyzing polarization-resolved photon statistics, effectively linking optical signatures to magnetic symmetries. By connecting measurable photon bunching patterns to the Raman structure factor, the study provides a diagnostic tool for characterizing phase transitions in Kitaev-Heisenberg models without direct matter probes. The work advances our ability to isolate higher-order scattering processes, offering new pathways for engineering material properties through cavity quantum electrodynamics.
Polarization-Resolved Photon Statistics of Cavity Quantum Materials
arXiv:2606.11550v2 Announce Type: replace-cross Abstract: By forming hybrid light-matter states, optical cavities offer a route for engineering material properties, however, unambiguously probing the effects of light-matter coupling remains difficult. Here, we show that the polarization-resolved statistics of photons transmitted through a cavity, measurable via $g^{(2)}$, provide one such diagnostic. By relating $g^{(2)}$ to matter correlation functions such as the Raman structure factor, we link photon bunching and antibunching to material properties. By applying this method to the stripy-to-antiferromagnetic transition in the Kitaev-Heisenberg spin model, we find that polarization-dependent patterns of bunching and antibunching encode the magnetic point-group symmetries of each phase and characterize the behavior at the phase boundary. Finally, we predict measuring $g^{(2)}$ for output photon pairs polarized orthogonal to the input field will isolate higher-order light-matter scattering processes that probe higher-order material correlations.
Abstract:By forming hybrid light-matter states, optical cavities offer a route for engineering material properties, however, unambiguously probing the effects of light-matter coupling remains difficult. Here, we show that the polarization-resolved statistics of photons transmitted through a cavity, measurable via $g^{(2)}$, provide one such diagnostic. By relating $g^{(2)}$ to matter correlation functions such as the Raman structure factor, we link photon bunching and antibunching to material properties. By applying this method to the stripy-to-antiferromagnetic transition in the Kitaev-Heisenberg spin model, we find that polarization-dependent patterns of bunching and antibunching encode the magnetic point-group symmetries of each phase and characterize the behavior at the phase boundary. Finally, we predict measuring $g^{(2)}$ for output photon pairs polarized orthogonal to the input field will isolate higher-order light-matter scattering processes that probe higher-order material correlations.
Mesoscale and Nanoscale Physics (cond-mat.mes-hall); Strongly Correlated Electrons (cond-mat.str-el); Optics (physics.optics); Quantum Physics (quant-ph)
arXiv:2606.11550 [cond-mat.mes-hall]
(or arXiv:2606.11550v2 [cond-mat.mes-hall] for this version)
Phys. Rev. B 114, 165130 (2026)
https://doi.org/10.1103/34vt-61w5 DOI(s) linking to related resources
Text integral sub licența deschisă a publicației · 164 cuvinte
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Polarization-Resolved Photon Statistics of Cavity Quantum Materials
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